What do you want to learnt? spanisch?
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Then madrid, in Barcelona speak catalan, and this is another language. Barcelona is nice and cool but they speak catalan mostly. Valencia is a nice place too, but a lot of people speak valenciano. With sea?? murcia, andalucia, cantabria, asturias. But if you want speak a very perfect spanich, then salamanca, valladolid...., inside the country. That is my opinion only.